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Author Pureur, P.; Sereni, J.G.; Schaf, J.
Title Specific heat and magnetic susceptibility in YNd alloys Type Journal Article
Year 1992 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 104 Issue 3 Pages (down) 1632-1634
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Abstract We report on the specific heat and dc magnetic susceptibility measurements of the YNd 4.5, 6.8 and 9.0 at % alloys. These systems present long-range SDW order just below the critical temperature. For temperatures well below T(C), the spin glass type of behavior is manifest. An interpretation is given in terms of a disorder- and frustration-induced breaking of the SDW coherence into small domains.
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ISSN 0304-8853 ISBN Medium
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Notes ISI:A1992HH32800067 Approved no
Call Number BT @ hernan @ Serial 115
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Author Braghta, A.; Schmerber, G.; Derory, A.; Sereni, J.G.; Kappler, J.P.
Title Magnetic and thermal properties of Ce2Pd2Sn Type Journal Article
Year 2008 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 320 Issue 6 Pages (down) 1141-1145
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Abstract X-ray diffraction, susceptibility and specific heat studies on ternary Ce2Pd2Sn intermetallic compound and on its isostructural nonmagnetic compound La2Pd2Sn are reported. On Ce2Pd2Sn in absence of magnetic field, we confirm the existence of two magnetic transitions at T-N = 4.8K (antiferromagnetic transition) and T-C = 2.2K (ferromagnetic transition) and the specific heat results, measured down to 0.5 K, allow to recognize the transition at 2.2K as a first-order transition. A description based on molecular field calculations for the S = 1/2 resonant level model leads to a characteristic Kondo T-K of about 3K. (C) 2007 Elsevier B.V. All rights reserved.
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Notes ISI:000254416300060 Approved no
Call Number BT @ hernan @ Serial 49
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Author Tovar, M.; Sereni, J.G.; Pedrazzini, P.; Caneiro, A.; Prado, F.; Butera, A.; Causa, M.T.
Title Magnetization and specific heat of La doped Sr2FeMoO6 Type Journal Article
Year 2004 Publication JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS Abbreviated Journal J. Magn. Magn. Mater.
Volume 272 Issue Pages (down) 857-858
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Abstract We present high-temperature magnetization and low-temperature specific heat measurements performed on the electron doped double perovskite Sr1.7La0.3FeMoO6. We have obtained the electronic contribution to C-p, gamma = 11.5(5) mJ/mol K-2. The electronic susceptibility, derived from the magnetic measurements in the paramagnetic regime (T > T-c = 390K), was chi(e)(0) =(4.9 +/- 1.5) x 10(-4) emu/mol. Anti ferromagnetic coupling between localized and itinerant moments was inferred from the data, with a coupling constant lambda = -(475 +/- 50)mol/emu, that results in a ferromagnetic-like Curie-Weiss susceptibility with Theta = 390(5) K. These results are compared with those obtained for the undoped material. (C) 2003 Published by Elsevier B.V.
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Notes ISI:000222236700045 Approved no
Call Number BT @ hernan @ Serial 63
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Author Betancourth, D.; Facio, J.I.; Pedrazzini, P.; Jesus, C.B.R.; Pagliuso, P.G.; Vildosola, V.; Cornaglia, P.S.; García, D. J.; Correa, V. F.
Title Low Temperature magnetic properties of GdCoIn5 Type Journal Article
Year 2015 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 374 Issue Pages (down) 744-747
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Abstract A comprehensive experimental and theoretical study of the low temperature properties of GdCoIn5 was performed. Specific heat, thermal expansion, magnetization and electrical resistivity were measured in good quality single crystals down to 4He temperatures. All the experiments show a second-order-like phase transition at 30 K probably associated with the onset of antiferromagnetic order. The magnetic susceptibility shows a pronounced anisotropy below T N with an easy magnetic axis perpendicular to the crystallographic ĉ-axis. Total energy GGA+U calculations indicate a ground state with magnetic moments localized at the Gd ions and allowed a determination of the Gd-Gd magnetic interactions. Band structure calculations of the electron and phonon contributions to the specific heat together with Quantum Monte Carlo calculations of the magnetic contributions show a very good agreement with the experimental data. Comparison between experiment and calculations suggests a significant anharmonic contribution to the specific heat at high temperature (View the MathML sourceT≳100K).
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Notes Approved no
Call Number BT @ victor.correa @ Serial 701
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Author Sereni, J.G.; Nieva, G.; Huber, J.G.; Braun, E.; Oster, F.; Bruck, E.; Roden, B.; Wohlleben, D.
Title Evidence for 4f-instability of dilute terbium in thorium Type Journal Article
Year 1987 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 63-64 Issue Pages (down) 597-599
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Abstract We have measured the specific heat of dilute Th1?xTbx alloys (0.44 < x < 2.15 a/o), which rises linearly between 0.4 and 0.9 K with a slope of ?C/T ? 450 mJ/K2molTb followed by a Schottky anomaly with a maximum near 3.8 K. The high temperature ??T product was found to be 4% lower than that of Tb3+. The resistivity shows no minimum at low temperatures. Discussion is made in terms of non-integral valence of Tb.
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Notes ISI:A1987G356900173 Approved no
Call Number BT @ hernan @ Serial 129
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Author Facio, J.I.; Betancourth, D.; Cejas Bolecek, N.R.; Jorge, G.A.; Pedrazzini, P.; Correa, V.F.; Cornaglia, P.S.; Vildosola, V.; García D.J.
Title Lattice specific heat for the RMIn5 (R=Gd, La,Y; M=Co, Rh) compounds: Non-magnetic contribution subtraction Type Journal Article
Year 2016 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 407 Issue Pages (down) 406-4011
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Notes Approved no
Call Number BT @ victor.correa @ Serial 730
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Author Sereni, J.G.; Kappler, J.P.
Title Magnetic and thermal properties of CeCu Type Journal Article
Year 1992 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 109 Issue 2-3 Pages (down) 349-352
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Abstract Magnetic susceptibility, high field magnetization and specific heat measurements on CeCu are presented. An antiferromagnetic transition is observed at T(N) = 313 K, with some evidences of low dimensionality of the order parameter. The saturation magnetization. M(s) = 1.16-mu(B), implies that the crystalline electric field (CEF) ground state doublet is strongly magnetic, in agreement with the low temperature Curie constant C = 0.46 emu K/mol. In the high temperature limit (T > 50 K), the obtained Curie constant is C = 0.65 emu K/mol, which suggests an overall CEF splitting larger than 200 K. The entropy gain at the magnetic transition is 72% of the expected R in 2. The missing entropy is related to a specific heat anomaly with a maximum at approximately 13 K, which is attributed to magnetic fluctuations in the Ce chains. The transition temperature and the high temperature broad maximum in the specific heat are weakly affected by an applied magnetic field of 1 T.
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Notes ISI:A1992HP06000034 Approved no
Call Number BT @ hernan @ Serial 112
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Author Kappler, J.P.; Schmerber, G.; Sereni, J.G.
Title Magnetic and thermal properties of Ce5Rh3 Type Journal Article
Year 1992 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 115 Issue 2-3 Pages (down) 241-244
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Abstract Magnetic susceptibility, high field magnetization and specific heat measurements on Ce5Rh3 are reported. Two antiferromagnetic transitions are observed at T(N)=4.5 K and T(N)'=2.6 K. The magnetization curve at 1.5 K reveals a nontrivial magnetic structure in this compound, with a saturation magnetization of 0.72mu(B). The high temperature Curie constant (0.64 emu K/mol), the Curie-Weiss constant (THETA(p)=-45 K) and the entropy related with the magnetic transitions (DELTAS(m)=0.8 R In 2) indicate the presence of a Kondo-type component in the ground state of Ce5Rh3.
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Notes ISI:A1992JV02200022 Approved no
Call Number BT @ hernan @ Serial 111
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Author SERENI, J.G.
Title The role of “p-like” orbitals in Ce valence instabilities Type Journal Article
Year 1985 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 47-48 Issue FEB Pages (down) 228-230
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Abstract From the analysis of spectroscopical data of atomic Ce, the [f(dsp)] configuration is found to be the least energetic when the metallization enthalpy is taken into account. The p-character of the band in Ce IV compounds is discussed and the p-f hybridization proposed.
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Notes ISI:A1985AKL5200061 Approved no
Call Number BT @ hernan @ Serial 131
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Author Pureur, P.; Fraga, G. L.; Brandao, D. E.; Caudron,R.; Safa, H.; Nieva, G.
Title Specific heat measurements in scandium-rare earth anisotropic spin glasses Type Journal Article
Year 1987 Publication Journal of Magnetism and Magnetic Materials Abbreviated Journal J. Magn. Magn. Mater.
Volume 68 Issue 2 Pages (down) 213-217
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Abstract We report on specific heat measurements at low temperature of the anisotropic spin glass alloys ScDy 3 at%, ScEr 4.25 at% and ScEr 10 at%. We find that at the lowest temperature range the data indicate the occurrence of an anisotropy induced gap around zero frequency in the density of states of the magnetic excitations. Moreover, some of our specific heat curves present a maximum coinciding with Tg, raising thus the question of thermal signs for a spin glass phase transition in anisotropic systems.
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Notes Approved no
Call Number BT @ gnieva @ Serial 425
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