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Wuyts, B., E. Osquiguil, M. Maenhoudt, S. Libbrecht, Z. X. Gao, and Y. Bruynseraede. "Relation between the Hall angle slope and the carrier density in oxygen-depleted YBa2Cu3Ox films." Physica C: Superconductivity and its applications 222, no. 3-4 (1994): 341–348.
Abstract: A detailed study of the Hall angle cot?H in YBa2Cu3Ox epitaxial thin films with various oxygen contents clearly shows the existence of a linear relation between the slope of cot?H versus T2 and the carrier density. The zero-temperature intercept C=cot?H(T=0 K) and the mobility at room temperature change substantially for an oxygen content x?6.6, indicating that both effects are closely related.
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Wuyts, B., E. Osquiguil, M. Maenhoudt, S. Libbrecht, Z. X. Gao, and Y. Bruynseraede. "Influence of the oxygen content on the normal-state Hall angle in YBa2Cu3Oxn films." Physical Review B 47, no. 9 (1993): 5512–5515.
Abstract: We report on measurements of in-plane resistivity ?ab(T) and Hall coefficient RH(T) in c-axis-oriented oxygen-deficient YBa2Cu3Oxn thin films. Independent of the changes induced in RH(T) and ?ab(T) by the oxygen depletion, a quadratic temperature dependence is observed for the Hall angle ?H. The slope of cot?H versus T2 decreases as the oxygen content xn is reduced and saturates in the Tc(xn)=60 K plateau region. The results are discussed in the framework of the two-dimensional Luttinger liquid theory as proposed by Anderson.
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Wuyts, B., M. Maenhoudt, S. Libbrecht, Z. X. Gao, E. Osquiguil, V. V. Moshchalkov, and Y. Bruynseraede. "Linear relation between the Hall angle slope and the carrier density in YBa2Cu3Ox films." Physica C: Superconductivity and its applications 235-240, no. PART 2 (1994): 1369–1370.
Abstract: A universal relation cot?H??{variant}/RHB = ?T2 + C for the Hall angle ?H has been experimentally observed served in a wide variety of high-Tc systems. In contrast to the linear temperature dependence of the resistivity ?{variant} or the inverse Hall coefficient R-1H, the T2-dependence of cot?H remains valid in under- and overdoped systems. We present a systematic study of cot?H(T) in oxygen deficient epitaxial YBa2Cu3Ox thin films. We find evidence for a linear relation between ?, the slope of cot?H versus T2, and the carrier concentration. Moreover, we find a steep increase in the intercept C = cot?H (T = 0) below x ? 6.6.
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Wuyts, B., Z. X. Gao, S. Libbrecht, M. Maenhoudt, E. Osquiguil, and Y. Bruynseraede. "Growth of particle-free YBa2Cu3O7 films by off-axis sputtering." Physica C: Superconductivity and its applications 203, no. 3-4 (1992): 235–239.
Abstract: The preparation of good YBa2Cu3O7 thin films is often hindered by the production of non-stoichiometric particles which degrade the superconducting properties of the layer. A systematic study of films prepared by off-axis single target magnetron sputtering shows that the presence of copper-rich particles dramatically decreases the critical current density but does not affect the critical temperature. The formation of these particles can be avoided by carefully adjusting the position of the substrate with respect to the target. Films without off-stoichiometric particles have excellent superconducting properties.
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Vanacken, J., S. Libbrecht, M. Maenhoudt, C. Van Haesendonck, E. Osquiguil, and Y. Bruynseraede. "The magnetic moment relaxation in oxygen-deficient YBa2Cu3Ox." Physica C: Superconductivity and its applications 197, no. 1-2 (1992): 9–14.
Abstract: The magnetic moment relaxation in polycrystalline YBa2Cu3Oxmaterial has been studied using zero-field-cooled measurements. The temperature dependence of the relaxation rate shows a field-dependent maximum. When the oxygen content is reduced, the maximum shifts towards lower temperatures. This shift is directly related to a decrease of the intragrain critical current density in the oxygen-deficient material, inducing a decrease of the field H* for complete flux penetration. The characteristic activation energies for depinning in the oxygen-deficient material are below 20 meV.
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Osquiguil, E., M. Maenhoudt, B. Wuyts, Y. Bruynseraede, D. Lederman, and I. K. Schuller. "Photoexcitation and oxygen ordering in YBa2Cu3Ox films." Physical Review B 49, no. 5 (1994): 3675–3678.
Abstract: We report on the photoinduced enhancement of the critical temperature ?Tc and the in-plane conductivity ??ab measured in a c-axis-oriented YBa2Cu3Ox film as a function of oxygen concentration (6.4?x?7). Both ?Tc and ??ab decrease with the oxygen content, display a plateaulike behavior for 6.6?x?6.75, and become zero at x=7. This dependence of ?Tc on x is similar to that observed for the Tc enhancement due to ordering effects in oxygen-deficient YBa2Cu3Ox single crystals. We propose that the persistent photoinduced changes in YBa2Cu3Ox films are due to photoassisted oxygen ordering.
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Osquiguil, E., M. Maenhoudt, B. Wuyts, Y. Bruynseraede, D. Lederman, G. Nieva, J. Guimpel, and I. K. Schuller. "Photoexcitation effects in YBa2Cu3Ox." Journal of Alloys and Compounds 195, no. C (1993): 667–670.
Abstract: We show through photoexcitation experiments carried out on YBa2Cu3Ox c-axis oriented films that photoinduced phenomena are not restricted to insulating samples. Superconducting films with critical temperatures varying between 2 K and 40 K show a clear enhancement of the superconducting transition after illumination. The increase in Tc is accompanied by a corresponding decrease in the resistivity ?, and an increase in the Hall coefficient RH, indicative of an increased carrier density. Furthermore, the carrier mobility is also affected by illumination.
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Osquiguil, E., M. Maenhoudt, B. Wuyts, and Y. Bruynseraede. "Controlled preparation of oxygen deficient YBa2Cu 3Ox films." Applied Physics Letters 60, no. 13 (1992): 1627–1629.
Abstract: We describe a simple method based on the oxygen pressure-temperature phase diagram to prepare oxygen deficient YBa2Cu3Ox thin films. Systematic critical temperature and x-ray diffraction experiments clearly show that films with different oxygen contents (6.6?x?7) are obtained in a controlled, reproducible, and reversible way.
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Osquiguil, E., Z. X. Gao, M. Maenhoudt, B. Wuyts, S. Libbrecht, and Y. Bruynseraede. "YBa2Cu3Ox: A natural multilayer system with tunable anisotropy." Journal of Physics: Condensed Matter 5, no. 33 A (1993).
Abstract: The authors report on magnetoresistivity rho ab( theta ,H,T) measurements below Tc in YBa2Cu3Oxn films with differing oxygen content x. The observed variations in the angular and field dependence of rho ab with reduced x indicate a gradual dimensional crossover from an anisotropic 3D to a quasi-2D behaviour. The increasing anisotropy is related to a decrease of the coupling between the Cu2O2 bilayers when oxygen is removed from the Cu1Ox chain-planes.
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Nieva, G., E. Osquiguil, J. Guimpel, M. Maenhoudt, B. Wuyts, Y. Bruynseraede, M. B. Maple, and I. K. Schuller. "Photoinduced enhancement of superconductivity." Applied Physics Letters 60, no. 17 (1992): 2159–2161.
Abstract: We show clear and conclusive experimental evidence for the enhancement of superconductivity in GdBa2Cu3Ox and YBa 2Cu3Ox thin films by photoexcitation. Upon laser illumination the critical temperature increases while the resistivity of the material decreases. The relaxation back to the original state is very slow, of the order of days at room temperature. The existence of this effect opens the possibility of fabricating weak-link devices with in situ tunable superconducting characteristics.
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